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The significance of the brand new inter-BrnNTE Br⋯O relations are after that backed by evaluating the new phosphorescence out of crystalline BrnNTE thereupon of your own spreading particles within the poly(methyl web site methacrylate) (PMMA, Mw ∼996 kDa; dos wt% doping). The newest tight polymer matrix is anticipated in order to constrain the fresh molecular action in the room-temperature however, disrupt inter-BrnNTE Br⋯O halogen ties. The new phosphorescence spectra away from Br1NTE stayed similar in both ecosystem (Fig. 2), appearing that triplet rust inside Br1NTE is simply inherent to the newest monomeric molecule.

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The interest rate constants kobs and kTT (red to have rac-BINAP and you may bluish for R-BINAP) is deduced from the investigation fit with Eq. B The fresh literary works said decay duration of lime-red-colored low-thing RTP dust (to possess information on per count, delight discover More Dining table 3 and A lot more Fig. 20)39,40,41,42,43,forty-a few,forty-four,46. Spectral brief improvement your PL spectrum for (c) rac-BINAP and you can (d) R-BINAP in the single crystal measured on the variation decrease time which have a great home thickness away from 200 μs.